2022-2023 / CHIM0697-1

Heterogeneous catalysis

Duration

20h Th, 20h Pr, 10h Proj.

Number of credits

 Master of Science (MSc) in Chemical and Materials Engineering5 crédits 
 Master of Science (MSc) in Engineering Physics5 crédits 

Lecturer

Nathalie Job

Language(s) of instruction

English language

Organisation and examination

Teaching in the first semester, review in January

Schedule

Schedule online

Units courses prerequisite and corequisite

Prerequisite or corequisite units are presented within each program

Learning unit contents

The course aims at developing the concepts required to use heterogeneous catalysts in various chemical processes. It contains the following concepts:  




  • Catalyst definition, types of catalysts.
  • History of catalysis - historical processes.
  • Industrial applications: relationship between process, reactor and catalyst;
  • Physical and chemical steps in heterogeneous catalysis (diffusion, adsorption, reaction, desorption);
  • Definition of catalytic sites - catalysis by metals, alloys and surface groups.
  • Conversion ratio, activity, selectivity, turnover number
  • Identification and counting of catalytic sites. catalyst characterization.
  • Nature and synthesis of supports and active phase. catalyst shaping.
  • Coupling between reaction and diffusion in porous catalysts (mass and heat transfers, efficiency factor, diffusional limitation
  • Deactivation
 

Learning outcomes of the learning unit

Master the concepts of catalyst preparation and characterization.

Be able to use a supported catalyst in a reactor and to determine the operating conditions (chemical vs. diffusional regime).

This course contributes to the learning outcomes I.1, I.2, II.1, II.2, III.1, III.2, III.4, IV.2, VI.1, VI.2, VII.1, VII.2, VII.3, VII.4, VII.5 of the MSc in biomedical engineering.


This course contributes to the learning outcomes I.1, I.2, II.1, II.2, III.1, III.2, III.4, IV.2, IV.3, IV.4, VI.1, VI.2, VII.1, VII.2, VII.3, VII.4, VII.5 of the MSc in chemical and material science engineering.


This course contributes to the learning outcomes I.1, I.2, II.1, II.2, III.1, III.2, III.2, III.4, IV.2, VI.1, VI.2, VII.1, VII.2, VII.3, VII.4, VII.5 of the MSc in engineering physics.

Prerequisite knowledge and skills

Corequis : CHIM0022-4 - Transport phenomena

 

or equivalent 

Planned learning activities and teaching methods

Theory lessons with numerous real examples about the preparation, characterization and use of catalysts.
  
Exercises about characterization data treatment and the study of reaction-mass transport coupling.

 
One group presentation (in English) on a predefined subject (relationship catalyst - process) as an exercise prior to flipped class. Flipped class will consist in one group presentation (in English) on a predefined subject (characterization technique) and writing of a report corresponding to the presentation. The slides and reports will constitue Chapter 7 of the course (flipped classroom).

Mode of delivery (face to face, distance learning, hybrid learning)

  • Lectures (theory), Autumn session (face-to-face).   
  • Practice, parallel to theoretical lectures (face-to-face).   
  • Language : English

Recommended or required readings

All teaching and practice material (slides and exercises) is available on the eCampus portal.

Recommended bibliography:

1.« Catalysis - an integrated approach », R.A. van Santen, P.W.N.M. van Leeuwen, J.A. Moulijn, B.A. Averill (Eds.), Elsevier, Amsterdam, 1999.

2.«  Synthesis of solid catalysts », K.P. de Jong (Ed.), Wiley-VCH, Weinheim, 2009.

3.« Catalyst preparation, Science and Engineering », J.R. Regalbuto (Ed.), CRC Press, Taylor & Francis Group, Boca Raton (FL), 2007.

4.« Mass tranfer in heterogeneous catalysis », C.N. Satterfield, MIT Press, Cambridge (MA) 1970.

5. « Concepts of modern catalysis and kinetics », I. Chorkendorff, J.W. Niemantsverdriet, Wiley, Weinheim, 2003 

Exam(s) in session

Any session

- In-person

written exam

Written work / report

Other : Oral presentation by groups of 2 students (inverse class)


Additional information:

  • Group presentation on a defined subejct (in English) during the theory lectures and writing of a report (10 pages maximum, English). The students may be questioned on any subject presented at the examination.  The presentation/report is mandatory: a students who fails in delivering the presentation and/or the report will not be admitted to the written examination.
 










  • Written examination on theory and practice (January).
 








  • Weighing ratios: personal presentation: 20%; written examination: 80%.
   

Work placement(s)

Organizational remarks

No remark

Contacts

Nathalie Job Department of Chemical Engineering Institut de Chimie - B6a   Tel. : 32-(0)4-366 35 37 e-mail : Nathalie.Job@uliege.be

Association of one or more MOOCs